Probing Spin Dynamics of 2D Excitons with Twisted Light

نویسندگان

چکیده

We propose a mechanism of intravalley spin-flip scattering in spin-valley coupled two dimensional systems by transferring momentum light into exciton center mass using optical vortex (OV) beams. By varying the dispersion topological charge OV beam, we demonstrate unique approach to control intra-valley rate excitons. From our photoluminescence measurements, that W-based TMDs can be tuned externally Variation intensity with charges shows crossover temperature (> 150 K), indicating competitions among time scales involving radiative recombination, scattering, and thermal relaxations. Our proposed technique utilizing structured beam open up new explore physics excitons 2D systems.

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ژورنال

عنوان ژورنال: ACS Photonics

سال: 2022

ISSN: ['2330-4022']

DOI: https://doi.org/10.1021/acsphotonics.2c00692